Abstract

N. Ph. Georgiades, E. S. Polzik and H. J. Kimble,
"Frequency Metrology by use of Quantum Interference,"
Opt. Lett. 21, 1688, (1996).

Quantum interference in the rate of two-photon excitation of the 6S1/2-->6P3/2-->6D5/2 transition in atomic cesium is exploited to demonstrate phase-sensitive frequency demodulation for an optical interval of +/- 12.5 THz. By thus using atoms as ultrafast nonlinear mixing elements, we suggest and analyze a new avenue of absolute comparisons of a dense set of frequencies over the range of 200-2000 nm.

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